Search results for "Transuranium element"
showing 10 items of 10 documents
Direct mass measurements and ionization potential measurements of the actinides
2019
Abstract The precise determination of atomic and nuclear properties such as masses, differential charge radii, nuclear spins, electromagnetic moments and the ionization potential of the actinides has been extended to the late actinides in recent years. In particular, laser spectroscopy and mass spectrometry have reached the region of heavy actinides that can only be produced only at accelerator facilities. The new results provide deeper insight into the impact of relativistic effects on the atomic structure and the evolution of nuclear shell effects around the deformed neutron shell closure at N = 152. All these experimental activities have also opened the door to extend such measurements t…
Trace analysis of plutonium in environmental samples by resonance ionization mass spectroscopy (RIMS)
1998
Resonance ionization mass spectroscopy (RIMS) is well suited for trace analysis of long-lived radioisotopes in environmental, biological and technical samples. By multiple resonant laser excitation and ionization of the elemental atoms under investigation, an extremely high element selectivity can be achieved. In addition, isotope selectivity is obtained by subsequent mass analysis. The excellent sensitivity results from the large atomic cross-sections in the excitation–ionization process and the good detection efficiency for ions. The element selectivity of RIMS allows a simplified procedure for the chemical preparation of the samples compared to the requirements of thin sources for α-spec…
Criteria for the Discovery of Chemical Elements
1976
The availability of suitable heavy-ion accelerators should make it possible to synthesize and identify additional heavy transuranium elements. Criteria for adequate proof that a new element has been synthesized or found in nature and identified are suggested. The basic criterion must be the proof that the atomic number of the new element is different from the atomic numbers of all previously known elements. Chemical identification constitutes an ideal proof; the procedure must be valid for application to individual atoms in an unequivocal manner. Also satisfactory is the identification of characteristic x rays in connection with the decay of the isotope of the new element. This is likely to…
Recent applications of the JYFL gas-filled recoil separator
1997
Abstract The gas-filled recoil separator RITU at the Department of Physics, University of Jyvaskyla (JYFL) was constructed in 1992–1993, and the first experiments were performed in late 1993. RITU differs from other gas-filled separators by having a vertically focusing quadrupole magnet in front of the separating dipole for better matching with the dipole acceptance. New results from RITU include the discovery of 13 previously unpublished isotopes of At, Rn, Fr, Ra, Ac and Th, while experiments in the transuranium region have also been made. Illustrative examples from these studies together with results on background properties, efficiency of separation, and other performance data will be p…
In-beam spectroscopy using the JYFL gas-filled magnetic recoil separator RITU
2003
The techniques of recoil-gating and recoil-decay tagging have been employed at Jyvaskyla to perform in-beam γ-ray and electron spectroscopy studies of heavy nuclei. The JUROSPHERE γ-ray array and the SACRED electron spectrometer have been placed at the target position of the JYFL gas-filled recoil separator recoil ion transport unit (RITU). The RITU separator has been used to collect the recoils of interest and separate them from beam particles and fission products. At the focal plane a detector system consisting of time-of-flight and implantation detectors has been used for further event identification. The method and some highlights from the results in the lead region close to the proton …
The impact of the properties of the heaviest elements on the chemical and physical sciences
2012
Abstract The unique role of the heaviest elements in chemical and physical sciences is discussed. With the actinide series (Z = 90-103) and the superactinide series (Z = 122-155), the heaviest elements have significantly shaped the architecture of the Periodic Table of the elements. Relativistic effects in the electron shells of the heaviest elements change the chemical properties in a given group in a non-linear fashion. Relativistically stabilized sub-shell closures give rise to a new category of elements in the Periodic Table: volatile metals. The prototype for this property is element 114 which, due to the relativistic stabilization of its 7s2 7p2 1/2 electron configuration, is volatile…
Syntheses of transuranium isotopes with atomic numbers Z≤ 103 in multi-nucleon transfer reactions
2015
Abstract In Section 1 we will discuss multi-nucleon transfer reactions with light heavy ions, which can be thought of as competing with complete fusion at higher impact parameters. Quasi-elastic and multi-nucleon transfer reactions with the heaviest projectiles will be discussed in Section 2 . In Section 3 we will cover recent developments focusing on theoretical predictions of cross sections of superheavy nuclei, cover some new possibilities and look into the existing experimental challenges.
SHIPTRAP—a capture and storage facility for heavy radionuclides at GSI
2002
Abstract SHIPTRAP will be an ion-trap facility for heavy radionuclides delivered from SHIP. Ion traps are a perfect instrument for precision measurements since the ions can be cooled to an extremely small phase space and can be stored for a very long time. In addition one can achieve very high purity by removing contaminant ions. SHIPTRAP will extend the possibilities of measurements in traps to transuranium nuclides and provide cooled and isobarically pure ion bunches.
First superheavy element experiments at the GSI recoil separator TASCA: The production and decay of element 114 in thePu244(Ca48,3-4n) reaction
2011
Experiments with the new recoil separator, Transactinide Separator and Chemistry Apparatus (TASCA), at the GSI were performed by using beams of Ca-48 to irradiate targets of Pb206-208, which led to the production of No252-254 isotopes. These studies allowed for evaluation of the performance of TASCA when coupled to a new detector and electronics system. By following these studies, the isotopes of element 114 ((288-291)114) were produced in irradiations of Pu-244 targets with Ca-48 beams at compound nucleus excitation energies around 41.7 and 37.5 MeV, demonstrating TASCA's ability to perform experiments with picobarn-level cross sections. A total of 15 decay chains were observed and were as…
Gas-filled separators – An overview
2003
Gas-filled recoil separators have been used in nuclear physics studies since the early fifties. Most notably, they have found use in the separation of evaporation residues of heavy and very heavy elements from unwanted background. Gas-filled separators, alone or coupled to a detector array, offer an efficient, fast, compact and relatively inexpensive solution for nuclear structure studies. A new application is the use of a gas-filled device as a pre-separator in the study of chemical properties of the heaviest elements. Other uses include systematic study of fusion evaporation cross sections and accelerator mass spectrometry. In this contribution, an overview on gas-filled recoil separators…